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Hokama, Tomonori; Kimura, Masanori; Togawa, Orihiko
JAEA-Research 2023-010, 57 Pages, 2024/02
JAEA-Research-2023-010.pdf:3.29MB
In the case of a nuclear accident, itis planned to perform simple measurement of radioactive iodine radioactivity in the thyroid of residents. The screening level for simple measurement is set at 0.20 
Sv/h as a reference, and it is required to be reviewed appropriately according to the situation such as a nuclear accident. However, a specific method for reviewing the screening level is not shown. When reviewing the screening level, it is important to take into account factors related to the feasibility of simple measurement, such as the judgment level for internal exposure dose of the thyroid and the duration of the measurement period. In this study, we organized the derivation process of 0.20 Sv/h, which was set as the reference for screening level, and considered the feasibility of the reviewing of screening level. We calculated the relationship between the judgment level and the duration of simple measurement for each screening level, ranging from 0.025 to 0.50 Sv/h. Then, the feasibility of the reviewing of screening level was considered. It was found that reviewing the screening level is technically feasible, provided that the judgment level and the duration of simple measurement are appropriate. However, assuming that simple measurement will be performed in an actual nuclear accident, we assessed that it would be reasonable to review the screening level within the range of 0.030 to 0.20 Sv/h, in a situation where the duration of simple measurement must be extended.
Onuki, Toshihiko*; Ye, J.*; Kato, Tomoaki; Liu, J.; Takano, Masahide; Kozai, Naofumi; Utsunomiya, Satoshi*
Environmental Science; Processes & Impacts, 25(7), p.1204 - 1212, 2023/07
Times Cited Count：0 Percentile：0(Chemistry, Analytical)To elucidate chemical forms of Cs and I in microparticles produced via the Fukushima Daiichi Nuclear Power Plant accident and released into the atmosphere, we analyzed Cs and I in condensed vaporized particles (CVP) produced by melting experiments using nuclear fuel components containing CsI with concrete. CVPs consisted of many round particles containing Cs and I of diameters less than several tens of micrometers. Two kinds of particles were present: one containing large amounts of Cs and I, suggesting the presence of CsI, and the other containing small amounts of Cs and I with large Si contents. Most of CsI from both particles were dissolved in water. On the contrary, some fractions of Cs remained from the latter particles. These results suggest that Cs was incorporated in CVPs along with Si to form water low-soluble CVPs
sp. DN11 and its potential use for removal of radioiodine from contaminated aquifersSasamura, Seiya*; Onuki, Toshihiko*; Kozai, Naofumi; Amachi, Seigo*
Frontiers in Microbiology (Internet), 14, p.1162788_1 - 1162788_7, 2023/04
Times Cited Count：2 Percentile：79.73(Microbiology) sp. DN11 previously isolated from gasoline-contaminated groundwater contained a gene cluster involved in bacterial iodate (IO
) respiration. This study determined if strain DN11 performed iodate respiration and assessed its potential use to remove and sequester radioactive iodine (
I) from subsurface contaminated aquifers. Strain DN11 grew anaerobically with iodate as the sole electron acceptor. After the growth of strain DN11 on iodate, silver-impregnated zeolite was added to the spent medium to remove iodide from the aqueous phase. In the presence of 200 M iodate as the electron acceptor, more than 98% of iodine was successfully removed from the aqueous phase. These results suggest that strain DN11 is potentially helpful for bioaugmentation of I-contaminated subsurface aquifers.
-CO mixed-gas reaction in inductively coupled plasma tandem quadrupole mass spectrometryMatsueda, Makoto; Aoki, Jo; Koarai, Kazuma; Terashima, Motoki; Takagai, Yoshitaka*
Analytical Sciences, 38(11), p.1371 - 1376, 2022/11
Times Cited Count：2 Percentile：15.48(Chemistry, Analytical)The I analysis using ICP-MS is challenging caused by xenon-129 (Xe) and 
IH generated from excess stable isotope I. In this study, mass discrimination between iodine-129 (I) and interfering substances was achieved by inductively coupled plasma-tandem quadrupole mass spectrometry (ICP-MS/MS) with a dynamic reaction cell introduced a mixture gas of O and CO. As a result, the ratio of (background noise intensity at m/z 129)/I was 3.8 
10
and 10 mBq/L of I was analyzed without chemical separation in the presence of 100 mg/L stable I. Spiked tests with actual rainwater were performed, and obtained values were agreed with the spiked amounts.
Tanimura, Yoshihiko
FBNews, (548), p.1 - 5, 2022/08
In the situation of a severe nuclear accident, radioiodine monitoring in thyroid should be performed for a large number of people immediately after accident. The portable thyroid dose monitoring system with the radiation shield which can be used in a high dose rate condition has been developed. In this paper, the outline of the monitoring system and the performance test results using the system will be described.
Kato, Tomoaki; Kozai, Naofumi; Tanaka, Kazuya; Kaplan, D. I.*; Utsunomiya, Satoshi*; Onuki, Toshihiko
Journal of Nuclear Science and Technology, 59(5), p.580 - 589, 2022/05
Times Cited Count：4 Percentile：56.94(Nuclear Science & Technology)This study reports the effect of fulvic acids, which is a natural organic substance generally contained in groundwater, on the oxidation states of radioactive iodine anions (iodide and iodate). Iodide and iodate are contained in the contaminated water of the Fukushima Daiichi Nuclear Power Plant and supposed to be removed by activated carbon (AC) via adsorption. When fulvic acids does not exist in the experimental system, the adsorption of iodide on AC was less than that of iodate and their oxidation states after the adsorption were not changed. When fulvic acids existed, a fraction of the adsorbed iodate was reduced to iodide. This result indicates that the reduction of the adsorbed iodate progresses during the storage of the spent AC.
I/I and 
C records in a modern coral from Rowley Shoals off northwestern Australia reflect the 20th-century human nuclear activities and ocean/atmosphere circulationsMitsuguchi, Takehiro; Okabe, Nobuaki*; Yokoyama, Yusuke*; Yoneda, Minoru*; Shibata, Yasuyuki*; Fujita, Natsuko; Watanabe, Takahiro; Kokubu, Yoko
Journal of Environmental Radioactivity, 235-236, p.106593_1 - 106593_10, 2021/09
Times Cited Count：5 Percentile：35.21(Environmental Sciences)For a contribution to developing the usage of iodine-129 (I) as a tracer of deep-seated fluid, I/I and C were measured for annual bands (AD 1931-1991) of a modern coral collected from Northwestern Australia; the measurements were performed using the JAEA-AMS-TONO-5MV for I/I and an AMS facility of the University of Tokyo for C. Results indicate that both I/I and C distinctly increase from 1950s. The C increase can be ascribed to atmospheric nuclear tests, while the I/I increase is due to nuclear-fuel reprocessing as well as atmospheric nuclear tests. These results are in good agreement with previous studies, indicating that the I/I measurement by JAEA-AMS-TONO-5MV has been further developed.
Tanimura, Yoshihiko; Yoshitomi, Hiroshi; Nishino, Sho; Takahashi, Masa
Radiation Measurements, 137, p.106389_1 - 106389_5, 2020/09
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)A portable thyroid dose monitoring system has been developed at the Japan Atomic Energy Agency (JAEA) to assess the thyroid equivalent dose for workers and members of the public in a high dose rate environment. The background (B.G.) photon correction is required for an accurate measurement in a high dose rate environment at an early stage after a nuclear accident. We developed the B.G. photon correction method using cylindrical PMMA phantoms.
, an iodine source for the immobilisation of radioiodineJohnstone, E. V.*; Bailey, D. J.*; Lawson, S.*; Stennett, M. C.*; Corkhill, C. L.*; Kim, M.*; Heo, J.*; Matsumura, Daiju; Hyatt, N. C.*
RSC Advances (Internet), 10(42), p.25116 - 25124, 2020/07
Times Cited Count：3 Percentile：15.55(Chemistry, Multidisciplinary)Nishino, Sho; Tanimura, Yoshihiko; Yoshitomi, Hiroshi; Takahashi, Masa
Radiation Measurements, 134, p.106292_1 - 106292_5, 2020/06
Times Cited Count：4 Percentile：45.45(Nuclear Science & Technology)In the situation of a severe nuclear accident, radioiodine monitoring in thyroid should be performed for a large number of people immediately after accident. The portable thyroid dose monitoring system which can be used in a high dose rate condition is in development. In this presentation, the result of performance test using prototype model will be described.
Guo, B.*; Xiong, Y.*; Chen, W.*; Saslow, S. A.*; Kozai, Naofumi; Onuki, Toshihiko*; Dabo, I.*; Sasaki, Keiko*
Journal of Hazardous Materials, 389, p.121880_1 - 121880_11, 2020/05
Times Cited Count：43 Percentile：90.61(Engineering, Environmental)I impacted by atmospheric I releases from a spent nuclear fuel reprocessing plantOta, Masakazu; Terada, Hiroaki; Hasegawa, Hidenao*; Kakiuchi, Hideki*
Science of the Total Environment, 704, p.135319_1 - 135319_15, 2020/02
Times Cited Count：6 Percentile：30.02(Environmental Sciences)Land-surface transfers of I are modeled and incorporated into a land-surface model (SOLVEG-II), and the model was applied to the observed transfer of I at a vegetated field impacted by atmospheric releases of I from Rokkasho reprocessing plant during 2007 to investigate the importance of each I-transfer pathway. The model calculation revealed that contamination of leaves of wild bamboo grasses was mostly caused by foliar adsorption of I (81%) induced via wet deposition of I. Wet deposition of I was the main I-input to the soil, ten-fold the dry deposition of I; however, the deposition of I during 2007 was only 2% of the model-assumed I that pre-existed in the soil; indicating the importance of long-term accumulation of I in soils. The model calculation also revealed that root uptake of I, not methylation, control the long-term turnover of soil I.
bus FP results and single effect testingKnebel, K.*; Jokiniemi, J.*; Bottomley, D.
Journal of Nuclear Science and Technology, 56(9-10), p.772 - 789, 2019/09
Times Cited Count：7 Percentile：58.58(Nuclear Science & Technology)Revaporisation of the fission products deposited in the primary circuit of a reactor was identified as a possible late source of fission product release during a severe accident: eg. loss of coolant accident (LOCA). Subsequent testing has shown that revaporisation is very likely to occur given a breach of the reactor and is an important contributor for the source term release to the containment and biosphere. The first part reviews the revaporisation mechanisms of Cs and other volatile or semi-volatile fission products transported in the primary circuit that were derived from the Phebus FP and associated programmes. The second part examines the separate effects testing to determine the high temperature chemistry ofvolatile and semi-volatile fission products (I, Mo, Ru) and structural materials (Ag, B) as well as atmospheric effects which substantially affect the source term. Finally, it examines Cs data from reactor accident sites that is providing additional knowledge of longer-term fission product chemistry. The results have been summarised in the form of a table and schematic diagram. This accumulated knowledge and experience has important applications to minimising contamination during decommissioning and site remediation techniques, as well as improving SA simulation codes and raising nuclear safety.
I released from Fukushima Daiichi Nuclear Power Plant accident in the western North Pacific OceanSuzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya
JAEA-Conf 2018-002, p.103 - 106, 2019/02
To investigate the dynamics of radionuclides in the ocean released by the accident at Fukushima Daiichi Nuclear Power Plant (1F), vertical distributions of I at three stations in the western North Pacific was revealed. The 1F accident-derived I existed within the mixed layer at 3 stations. The maximum layer of the 1F accident-derived I existed at the depth of 370 m - 470 m at the most southern station. Considering the dissolved oxygen concentration and the current velocity arround the station, the maximum layer of the 1F accident-derived I would be fromed that I which existed in the surface seawater at other area of observation point was carried to the depth of 370 m - 470 m by the fast downward flow.
I in the seabed sediment off FukushimaOtosaka, Shigeyoshi; Sato, Yuhi*; Suzuki, Takashi; Kuwabara, Jun; Nakanishi, Takahiro
Journal of Environmental Radioactivity, 192, p.208 - 218, 2018/12
Times Cited Count：15 Percentile：48.31(Environmental Sciences)From August 2011 to October 2013, the concentration of iodine-129 (I) in the seabed sediment collected from 26 stations located within 160 km from the Fukushima Daiichi Nuclear Power Plant was estimated. The concentrations of I in seabed sediment off Fukushima in 2011 ranged between 0.02 and 0.45 mBq/kg. Although iodine is a biophilic element, the accident-derived radioiodine negligibly affects the benthic ecosystem. Until October 2013, a slightly increased activity of I in the surface sediment in the shelf-edge region (bottom depth: 200-400 m) was observed. The increase of the I concentrations in the shelf-edge sediments was affected by the (1) transport of I-bound particles from the land through rivers and (2) re-deposition of I desorbed from the contaminated coastal sediment to the shelf-edge sediments, which were considered to be dominant processes.
Shiotsu, Hiroyuki; Ito, Hiroto*; Ishikawa, Jun; Sugiyama, Tomoyuki; Maruyama, Yu
Proceedings of 11th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-11) (Internet), 6 Pages, 2018/11
I released from the Fukushima Daiichi Nuclear Power Plant in the Kuroshio and Oyashio current areasSuzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya
Marine Chemistry, 204, p.163 - 171, 2018/08
Times Cited Count：2 Percentile：10.86(Chemistry, Multidisciplinary)To investigate the penetration of radionuclides released from Fukushima Daiichi Nuclear Power Plant (FDNPP), depth profiles were revealed at Kuroshio current, transition, and Oyashio current areas. The FDNPP-derived I was found in surface layer at Oyashio current and transition areas and in sub-surface layer at Kuroshio current area. Moreover, it was found that the FDNPP-derived I/
Cs ratios in the Oyashio current and transition areas were higher than that in the FDNPP reactor. The higher FDNPP-derived I/Cs ratios suggest three potential mechanisms for the migration of radionuclides in the environment: (1) radioiodine was released more easily than radiocesium by the FDNPP accident, (2) I was supplied from the atmosphere by re-emitted I from contaminated areas around Fukushima, (3) leaked water that removed radiocesium reached the sampling stations. The FDNPP-derived I in sub-surface layer would be transported by the meander of the Kuroshio Extension current.
I concentrations in the air from pulse-height distribution observed by NaI(Tl) detector in monitoring postsYamada, Junya; Hashimoto, Makoto; Seya, Natsumi; Haba, Risa; Muto, Yasunobu; Shimizu, Takehiko; Takasaki, Koji; Yokoyama, Sumi*; Shimo, Michikuni*
Radioisotopes, 65(10), p.403 - 408, 2016/10
The purpose of this study is to develop a quick method for estimation of I concentrations in the air using data measured by monitoring posts. In this method, I concentrations were estimated by multiplying I count rates at the full-energy peak measured with a NaI(Tl) detector by a concentration conversion factor. The concentration conversion factor for monitoring posts in JAEA Oarai Center was calculated with an EGS5 Monte Carlo code. As a result, the concentration conversion factor for an infinite-air-source was 25.7 Bq/m
/cps.
Hemmi, Ko
Genshiryoku Bakkuendo Kenkyu (CD-ROM), 23(1), P. 113, 2016/06
no abstracts in English
Shibata, Keiichi
Journal of Nuclear Science and Technology, 52(9), p.1174 - 1185, 2015/09
Times Cited Count：4 Percentile：33.25(Nuclear Science & Technology)Neutron nuclear data on 6 isotopes of iodine have been evaluated for the next release of JENDL general purpose file in the energy region from 10
eV to 20 MeV. Except for 
I, the thermal capture cross sections were determined from a simplified formula. Unresolved resonance parameters were obtained for self-shielding calculations. On the other hand, a statistical model code CCONE was applied to calculate cross sections above the resolved resonance region. Coupled-channel optical-model potentials were employed for the interaction between neutrons and nuclei. The 
-ray strength functions for iodine isotopes were determined so as to reproduce measured -ray spectrum for I. The presently evaluated results are consistent with available experimental data, and found to be much better than the JENDL-4.0 evaluation. The evaluated data are compiled into ENDF formatted data files.
